Cooperative reaction chemistry derived from a borata-diene framework

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Cooperative reaction chemistry derived from a borata-diene framework.

The bifunctional frustrated BH(-)/B hydridoborate nucleophile/borane Lewis acid pair 6 is prepared starting from the borata-diene 3 by a sequence of sequential protonation/hydride attachment, followed by hydroboration with Piers' borane [HB(C6F5)2]. The trans-1,2-bifunctional system 6 reduced carbon monoxide eventually to the aldehyde product 10.

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ژورنال

عنوان ژورنال: Chemical Communications

سال: 2016

ISSN: 1359-7345,1364-548X

DOI: 10.1039/c5cc07954c